Well, then you can't go wrong with any of his pre-electric material, with specific focus on The Freewheelin' Bob Dylan and The Times They Are a Changin'. Personally, I'd go with Another Side of Bob Dylan (my favorite pre-electric album, though it isn't such a pissed-off album).
Bringing It All Back Home still finds him damning the man, and is a great album, to boot. Then there's the aforementioned Highway 61 Revisited, which, among many, many highlights, features the angry stomp of "Tombstone Blues," a song that's both country and punk fucking rock. Ya know, cow punk.